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This question already has an answer here:

Can I transfer 2 accounts into one. I have an account that has all my money. But I accidentally used another account and that one has all my status. Can I transfer them both into one?

marked as duplicate by galacticninja, Wrigglenite, Isuka, user1306322, Ave Sep 8 '16 at 20:50

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You can try contacting steam support. But you'll have to prove you own both of them and there's no guarantee.

  • I had friends try this. Support gave negative replies to them in all cases. – Ave Sep 8 '16 at 16:32
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No, you can't combine steam accounts.

You can buy items/games on one and gift/trade it to the other one though.

You can also try Steam Family Sharing.

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